Ferrimagnets are described by molecular field models, which operate by summing sublattice magnetic moments with Brillouin functions. They are commonly initialized with the fully saturated ("spontaneous") moment Ms(T), obtained by extrapolating the high-field portion of M(H) hysteresis curves to zero-field. However, the bulk polycrystalline ferrimagnetic samples used in our experiments were measured in their remanent state, so the directly observed moment Mr(T) can differ significantly from Ms(T), leading to model and experiment mismatches of up to ~3x. We derive a practical connection between Ms(T) from the molecular field model and the experimental Mr(T). Our approach introduces a correction factor β(T) = Mr/Ms derived from hysteresis curves of our sample that can be folded back into the molecular field fit. Applying this correction to polycrystalline terbium iron garnet yields good agreement between the modeled and measured magnetization in the relevant temperature range, especially near the compensation temperature, which is where the richest physics resides. In addition, the corrected model reproduces the measured neutron spin rotation of our samples that depend on the internal magnetization of the sample. This explicit treatment of the remanent state reconciles the molecular field model with measurements on actual rare-earth iron garnet targets, providing a backbone to the results of the NSR-Ferrimagnets collaboration and other exotic force-searching experiments using ferrimagnets.
                    Previous Article in event
            
                            
    
                    Next Article in event
            
                            Next Article in session
            
                    
                                                    
        
                    Reconciling Molecular Field Models with Magnetization Data in Ferrimagnetic Iron Garnets
                
                                    
                
                
                    Published:
29 October 2025
by MDPI
in The 4th International Online Conference on Materials
session Optical, Electric and Magnetic Materials and Their Characterization
                
                
                
                    Abstract: 
                                    
                        Keywords: Ferrimagnets; Rare-earth iron garnets; Molecular field models
                    
                
                
                
                
        
            