EventsThe 3rd International Online Conference on Nanomaterials
Published
This submission belongs to the session A. Synthesis, Characterization, and Properties of Nanomaterials of the event The 3rd International Online Conference on Nanomaterials
Published date
24 Apr, 2022
Academic Editor
author-avatarGuanying Chen
Citation
Maria Burdanova, Maksim Paukov, Georgy Ermolaev, Mikhail Tatmyshevskiy, Adilet Taksumakov, Gennady Komandin, Sergey Novikov, Davit Ghazaryan, Yongjia Zheng, Roman Romanov, Rong Xiang, Shohei Chiashi, Shigeo Maruyama, James Lloyd-Hughes, Broadband Optical and Terahertz Properties of Atomically Thin 1D van der Waals Heterostructures, in Proceedings of The 3rd International Online Conference on Nanomaterials, 25 April–10 May 2022, MDPI: Basel, Switzerland
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Broadband Optical and Terahertz Properties of Atomically Thin 1D van der Waals Heterostructures

Yongjia Zheng 3
Adilet Taksumakov 5
Gennady Komandin 6
Davit Ghazaryan 5
Rong Xiang 3
Shohei Chiashi 3
image
James Lloyd-Hughes 8
1. Center for Photonics and 2D Materials, Moscow Institute of Physics and Technology, 9 Institutsky Lane, 141700 Dolgoprudny, Russia, Russia
2. Institute of Solid State Physics of the Russian Academy of Sciences, Chernogolovka, 142432, Russia
3. Department of Mechanical Engineering, The University of Tokyo, Tokyo, 113-8656 Japan
4. Center for Photonics and 2D Materials, Moscow Institute of Physics and Technology, 9 Institutsky Lane, 141700 Dolgoprudny, Russia
5. Center for Photonics and 2D Materials, Moscow Institute of Physics and Technology, Institutskii Pereulok 9, 141700 Dolgoprudny, Russia
6. Prokhorov General Physics Institute of the Russian Academy of Sciences, Vavilov str. 38, 119991, Moscow
7. Moscow Institute of Physics and Technology (National Research University), Institutskii per. 9, 141701 Dolgoprudny, Moscow Region, Russia
8. University of Warwick, Department of Physics, Gibbet Hill Road, Coventry, CV4 7AL UK
Abstract

We examined the optoelectronic properties of atomically thin 1D van der Waals heterostructures comprising the single-walled carbon nanotubes (NT) wrapped by insulating BN NT layers and MoS2 NT outer layers (C@BN@MoS2NT). We will present the equilibrium properties of such materials (through optical absorption, transmission, reflection, ellipsometry, Raman scattering, THz spectroscopy, and XPS studies) along with the transmission electron microscopy measurements. Through all of these techniques, we evaluated intertube excitonic interactions in addition to the charge transport characteristics of a large area 1D heterostructure. In addition, non-equilibrium, ultrafast pump–probe spectroscopy across the visible and terahertz frequency ranges identified that, in the MoS2 nanotubes, excitons coexisted with a prominent population of free charges.

Keywords
nanotubes
van der Waals heterostructures
ultrafast
ellipsometry
terahertz
XPS
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