Thunderstorm electrification arises from complex interactions among cloud microphysics, dynamics, and charge separation processes. Lightning and surface electric-field measurements alone cannot fully resolve the three-dimensional electrical structure of convective storms. Cosmic-ray muons, owing to their high penetrating power, provide a complementary probe of electrified cloud regions. Here, we investigate an intense convective thunderstorm over southern India on 27 April 2020 using a multi-instrumental framework that combines directional muon observations from the GRAPES-3 telescope [1], surface electric-field measurements, lightning location network data, satellite observations, ERA5 reanalysis, and high-resolution WRF simulations. After correcting the muon data for atmospheric pressure and solar-induced anisotropy, we identify a transient ~0.5% decrease in muon flux from the Southeast direction during the storm's mature phase [2-3]. This directional deficit occurs concurrently with enhanced electric-field variability, peak lightning activity, and the development of a vigorous mixed-phase region conducive to non-inductive charge separation, as indicated by satellite observations and WRF simulations. The consistency in timing and direction among these independent datasets provides compelling evidence for a close linkage between thunderstorm electrification and secondary cosmic-ray particles. These results demonstrate the value of directional muon observations as an independent diagnostic of electrified thunderstorms and highlight the potential of multi-instrumental analyses for investigating storm-scale electrical processes.
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