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Early Hydrochemical Evolution of Groundwater Under Landfill Leachate Influence: Case of the Tangier Municipal Site
* 1, 2 , 1 , 2 , 1 , 1
1  Research and Development in Applied Geosciences Laboratory, FSTT, Abdelmalek Essaadi University, Tetouan, Morocco
2  Department of Engineering, University of Messina, Villaggio S. Agata, 98166 Messina, Italy
Academic Editor: Nicolò Colombani

Abstract:

This study evaluates short-term changes in groundwater quality around the new municipal landfill of Tangier, Morocco . In total, 10 sampling sites (8 wells and 2 surface waters) within 2 km were sampled in late summer 2023 (S-23) and late winter 2025 (F-25), alongside the flow gradient. Major ions (ICs), trace metals (ICP-OES) and field parameters were analyzed; data were converted to milliequivalents and quality-checked by ionic balance error (IBE).

S-23 samples were mostly fresh Ca–HCO₃/Cl waters (EC < 1,000 µS cm⁻¹; TDS < 500 mg L⁻¹). By F-25, downgradient wells evolved from Ca–Cl to mixed Ca–Na–Cl–SO₄ facies, with Cl⁻ accounting for > 70% of anions and Ca²⁺ contributing to 20–50% of cations; the Piper diamond collapses toward the strong acid corner. A PCA on major ions (meq L⁻¹) shows PC1 (80.9%) as a salinity/leachate axis, clearly separating F-25 downgradient waters (notably P3–P4–P8) from upgradient S-23 points. PC2 (10.8%) represents hardness vs. alkalinity (SO₄/Mg/Ca vs HCO₃). A simple two-endmember chloride mixing model estimates the leachate fraction fL increasing from (0.0–0.1 upgradient) to (0.2–0.5 at P3–P4) and (0.9–1.0 at P8). Paired Wilcoxon tests (n = 10) on Cl⁻/SO₄²⁻ show non-significant p-values (0.19–0.38), reflecting limited power, yet large effect sizes are captured by PCA, medians and fL. Heavy metal enrichments (e.g., Fe, Mn and Zn) co-locate with high fL and strong acid fractions.

Together, these lines of evidence indicate rapid salinization and leachate intrusion in less than 2 years along the downgradient axis. We outline a monitoring framework (quarterly sampling, sentinel wells P3–P4–P8, trigger thresholds on EC/Cl/SO₄ and IBE), and propose MODFLOW transport modeling constrained by the local stratigraphy and measured heads to forecast plume migration and guide mitigation (drainage capture, liner integrity checks and wellhead protection).

Keywords: Groundwater quality; Leachate contamination; Landfill impact; Piper diagram; Hydrogeochemistry

 
 
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